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Conversion of methane and carbon dioxide to higher value products / Vesna Havran in Industrial & engineering chemistry research, Vol. 50 N° 12 (Juin 2011) 

Public ISBD [article]  in Industrial & engineering chemistry research > Vol. 50 N° 12 (Juin 2011) . - pp. 7089-7100 Titre : Conversion of methane and carbon dioxide to higher value products Type de document : texte imprimé Auteurs : Vesna Havran, Auteur ; Milorad P. Dudukovic, Auteur ; Cynthia S. Lo, Auteur Année de publication : 2011 Article en page(s) : pp. 7089-7100 Note générale : Chimie industrielle Langues : Anglais (eng) Mots-clés : Carbon  dioxide Résumé : In this manuscript we address the efforts reported in the literature on direct conversion of methane and carbon dioxide into higher value products. The abundance of these two greenhouse gases makes them potentially useful for chemical syntheses. However, strong intramolecular bonds render both molecules chemically inert and thermodynamically stable. Thus, significant energy inputs as well as properly designed catalytic systems are required for their reactions. In addition to traditional catalytic processes, new alternative routes-such as photocatalytic conversion and dielectric barrier discharges—have been suggested. Figures of merit for comparison of various approaches have not yet been reported and are overdue. DEWEY : 660 ISSN : 0888-5885 En ligne : http://cat.inist.fr/?aModele=afficheN&cpsidt=24239022 [article] Conversion of methane and carbon dioxide to higher value products [texte imprimé] / Vesna Havran, Auteur ; Milorad P. Dudukovic, Auteur ; Cynthia S. Lo, Auteur . - 2011 . - pp. 7089-7100. Chimie industrielle Langues : Anglais (eng) in Industrial & engineering chemistry research > Vol. 50 N° 12 (Juin 2011) . - pp. 7089-7100 Mots-clés : Carbon  dioxide Résumé : In this manuscript we address the efforts reported in the literature on direct conversion of methane and carbon dioxide into higher value products. The abundance of these two greenhouse gases makes them potentially useful for chemical syntheses. However, strong intramolecular bonds render both molecules chemically inert and thermodynamically stable. Thus, significant energy inputs as well as properly designed catalytic systems are required for their reactions. In addition to traditional catalytic processes, new alternative routes-such as photocatalytic conversion and dielectric barrier discharges—have been suggested. Figures of merit for comparison of various approaches have not yet been reported and are overdue. DEWEY : 660 ISSN : 0888-5885 En ligne : http://cat.inist.fr/?aModele=afficheN&cpsidt=24239022