Dynamics of CO2 absorption and desorption processes in alkanolamine with cosolvent polyethylene glycol / Jun Li in Industrial & engineering chemistry research, Vol. 51 N° 37 (Septembre 2012)  

Public ISBD [article]  inIndustrial & engineering chemistry research > Vol. 51 N° 37 (Septembre 2012) . - pp. 12081–12088 Titre : Dynamics of CO2 absorption and desorption processes in alkanolamine with cosolvent polyethylene glycol Type de document : texte imprimé Auteurs : Jun Li, Auteur ; Chenjia You, Auteur ; Lifang Chen, Auteur Année de publication : 2012 Article en page(s) : pp. 12081–12088 Note générale : Industrial chemistry Langues : Anglais (eng) Mots-clés : Dynamics Absorption Résumé : To reduce the high energy consumption and equipment corrosion in conventional processes of CO2 capture with aqueous amine solutions, the mixed nonaqueous solvents of monoethanolamine (MEA), diethanolamine (DEA), and diglycolamine (DGA) with polyethylene glycol (PEG) as cosolvent were explored for CO2 capture. The dynamic experiments of CO2 absorption and desorption were carried out to evaluate the performance of the studied nonaqueous solutions. It demonstrated that the mixed solutions of amines and PEG exhibited higher CO2 cyclic capacity and regeneration efficiency compared with the only aqueous amine solutions. Especially, the solution of 3 mol/L DGA-PEG200 exhibits a high cyclic capacity of 0.438 mol CO2/mol DGA and a high regeneration efficiency of 94.6%, which indicates its great potential in industrial application. Moreover, the very low vapor pressure of PEG helps the mixed solution for CO2 capture with reduced corrosion, energy consumption, and environmental pollution. ISSN : 0888-5885 En ligne : http://pubs.acs.org/doi/abs/10.1021/ie301164v [article] Dynamics of CO2 absorption and desorption processes in alkanolamine with cosolvent polyethylene glycol [texte imprimé] / Jun Li, Auteur ; Chenjia You, Auteur ; Lifang Chen, Auteur . - 2012 . - pp. 12081–12088. Industrial chemistry Langues : Anglais (eng) in Industrial & engineering chemistry research > Vol. 51 N° 37 (Septembre 2012) . - pp. 12081–12088 Mots-clés : Dynamics Absorption Résumé : To reduce the high energy consumption and equipment corrosion in conventional processes of CO2 capture with aqueous amine solutions, the mixed nonaqueous solvents of monoethanolamine (MEA), diethanolamine (DEA), and diglycolamine (DGA) with polyethylene glycol (PEG) as cosolvent were explored for CO2 capture. The dynamic experiments of CO2 absorption and desorption were carried out to evaluate the performance of the studied nonaqueous solutions. It demonstrated that the mixed solutions of amines and PEG exhibited higher CO2 cyclic capacity and regeneration efficiency compared with the only aqueous amine solutions. Especially, the solution of 3 mol/L DGA-PEG200 exhibits a high cyclic capacity of 0.438 mol CO2/mol DGA and a high regeneration efficiency of 94.6%, which indicates its great potential in industrial application. Moreover, the very low vapor pressure of PEG helps the mixed solution for CO2 capture with reduced corrosion, energy consumption, and environmental pollution. ISSN : 0888-5885 En ligne : http://pubs.acs.org/doi/abs/10.1021/ie301164v

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