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Understanding riser and downer based fluid catalytic cracking processes by a comprehensive two-dimensional reactor model / Changning Wu in Industrial & engineering chemistry research, Vol. 48 N°1 (Janvier 2009) 

Public ISBD [article]  in Industrial & engineering chemistry research > Vol. 48 N°1 (Janvier 2009) . - p. 12-26 Titre : Understanding riser and downer based fluid catalytic cracking processes by a comprehensive two-dimensional reactor model Type de document : texte imprimé Auteurs : Changning Wu, Editeur scientifique ; Yi Cheng, Editeur scientifique ; Yong Jin, Editeur scientifique Année de publication : 2009 Article en page(s) : p. 12-26 Note générale : Chemical engineering Langues : Anglais (eng) Mots-clés : Two-dimensional  reactor  Fluid  catalytic  cracking Résumé : A two-dimensional reactor model incorporating hydrodynamics, mass balance, energy balance, and a 4-lump/14-lump kinetic model was established to simulate the riser and downer based fluid catalytic cracking (FCC) processes. The kinetic parameters of the 4-lump kinetic model were re-evaluated from the originally published experimental data for a more reliable description of the FCC process. The 14-lump kinetic model based on a molecular description of cracking and hydrogen transfer reactions was to include more details about the feedstock composition, reaction mechanisms, and the products distribution for a better understanding on the reactor performance for FCC process. This comprehensive model captured the key characteristics of the gas−solid reacting flows in the riser and downer, i.e., the uniformity of flow structures, the distinct backmixing behavior in the riser and downer, and the momentum and energy balances during the complex FCC reactions. The model predictions were first validated against industrial data from several literature sources and found to agree with each other reasonably well. Then, the simulations were carried out to fully understand the different reactor performances of riser and downer in the application of FCC refining processes. It can be concluded that the downer benefits from its advantages of the plug-flow nature and uniform flow structures, tending to have more products in the middle distillates, e.g., gasoline and light olefins, especially under high-severity operations. Better control of the reaction extent for increased selectivity to desired intermediate products would allow the use of downer reactors for the larger-scale practical applications in the FCC process, together with the valuable byproduction of light olefins. En ligne : http://pubs.acs.org/doi/abs/10.1021/ie800168x [article] Understanding riser and downer based fluid catalytic cracking processes by a comprehensive two-dimensional reactor model [texte imprimé] / Changning Wu, Editeur scientifique ; Yi Cheng, Editeur scientifique ; Yong Jin, Editeur scientifique . - 2009 . - p. 12-26. Chemical engineering Langues : Anglais (eng) in Industrial & engineering chemistry research > Vol. 48 N°1 (Janvier 2009) . - p. 12-26 Mots-clés : Two-dimensional  reactor  Fluid  catalytic  cracking Résumé : A two-dimensional reactor model incorporating hydrodynamics, mass balance, energy balance, and a 4-lump/14-lump kinetic model was established to simulate the riser and downer based fluid catalytic cracking (FCC) processes. The kinetic parameters of the 4-lump kinetic model were re-evaluated from the originally published experimental data for a more reliable description of the FCC process. The 14-lump kinetic model based on a molecular description of cracking and hydrogen transfer reactions was to include more details about the feedstock composition, reaction mechanisms, and the products distribution for a better understanding on the reactor performance for FCC process. This comprehensive model captured the key characteristics of the gas−solid reacting flows in the riser and downer, i.e., the uniformity of flow structures, the distinct backmixing behavior in the riser and downer, and the momentum and energy balances during the complex FCC reactions. The model predictions were first validated against industrial data from several literature sources and found to agree with each other reasonably well. Then, the simulations were carried out to fully understand the different reactor performances of riser and downer in the application of FCC refining processes. It can be concluded that the downer benefits from its advantages of the plug-flow nature and uniform flow structures, tending to have more products in the middle distillates, e.g., gasoline and light olefins, especially under high-severity operations. Better control of the reaction extent for increased selectivity to desired intermediate products would allow the use of downer reactors for the larger-scale practical applications in the FCC process, together with the valuable byproduction of light olefins. En ligne : http://pubs.acs.org/doi/abs/10.1021/ie800168x